PREPARATION OF LITHIUM ION CONDUCTOR GLASS-CERAMIC WITH HIGH CONDUCTIVITY FOR PRODUCING LITHIUM-AIR AND ALL-SOLID-STATE LITHIUM-ION BATTERIES

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ILLBEIGI M.; FAZLALI A.R.; KAZAZI M.; MOHAMMADI A.H.

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Paper Information

Journal: ADVANCED MATERIALS IN ENGINEERING (ESTEGHLAL) Year:2017 | Volume:36 | Issue:1 Page(s): 37-52

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Information Journal Paper

Title

PREPARATION OF LITHIUM ION CONDUCTOR GLASS-CERAMIC WITH HIGH CONDUCTIVITY FOR PRODUCING LITHIUM-AIR AND ALL-SOLID-STATE LITHIUM-ION BATTERIES

Author(s)

ILLBEIGI M. | FAZLALI A.R. | KAZAZI M. | MOHAMMADI A.H. | Issue Writer Certificate

Keywords

SOLID ELECTROLYTEQ2

NASICON-TYPE GLASS-CERAMICQ2

LITHIUM ION CONDUCTORQ2

LITHIUM-AIR BATTERYQ2

ALL-SOLID-STATE BATTERYQ2

Abstract

In this research, new LITHIUM ION CONDUCTOR glass-ceramics with NASICON-type structure (Li1+x+yAlxCryGe2-x-y (PO4)3, x+y=0.5) were synthesized using melt-quenching method and converted to glass-ceramics through heat treatment. Influence of addition of different concentrations of aluminum and chromium in LiGe2(PO4)3 glass-ceramic was investigated for ionic conduction improvement. Substitution of Ge4+ions in NASICON structure by Al3+ and Cr3+ions induced more Li+ions in A2 vacant sites to obtain charge balance and also changed the unit cell parameters. These two factors led to ionic conductivity improvement of synthesized glass-ceramics. The glass-ceramics were characterized and the amorth structures were investigated by X-ray Diffraction (XRD), Field Emission Scanning Electron Microscopy (FESEM), Energy-Dispersive X-ray spectroscopy (EDX), Differential Scanning Calorimetry (DSC) and Complex Impedance Spectroscopy (CIS). The highest lithium ion conductivity of 8.82´10-3 S/cm was obtained for x=0.4 and y=0.1 (Li1.5Al0.4Cr0.1Ge1.5 (PO4)3) crystallized at 850oC for 8 h with minimum activation energy of 0.267 eV.

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APA: Copy

ILLBEIGI, M., FAZLALI, A.R., KAZAZI, M., & MOHAMMADI, A.H.. (2017). PREPARATION OF LITHIUM ION CONDUCTOR GLASS-CERAMIC WITH HIGH CONDUCTIVITY FOR PRODUCING LITHIUM-AIR AND ALL-SOLID-STATE LITHIUM-ION BATTERIES. ADVANCED MATERIALS IN ENGINEERING (ESTEGHLAL), 36(1 ), 37-52. SID. https://sid.ir/paper/163285/en

Vancouver: Copy

ILLBEIGI M., FAZLALI A.R., KAZAZI M., MOHAMMADI A.H.. PREPARATION OF LITHIUM ION CONDUCTOR GLASS-CERAMIC WITH HIGH CONDUCTIVITY FOR PRODUCING LITHIUM-AIR AND ALL-SOLID-STATE LITHIUM-ION BATTERIES. ADVANCED MATERIALS IN ENGINEERING (ESTEGHLAL)[Internet]. 2017;36(1 ):37-52. Available from: https://sid.ir/paper/163285/en

IEEE: Copy

M. ILLBEIGI, A.R. FAZLALI, M. KAZAZI, and A.H. MOHAMMADI, “PREPARATION OF LITHIUM ION CONDUCTOR GLASS-CERAMIC WITH HIGH CONDUCTIVITY FOR PRODUCING LITHIUM-AIR AND ALL-SOLID-STATE LITHIUM-ION BATTERIES,” ADVANCED MATERIALS IN ENGINEERING (ESTEGHLAL), vol. 36, no. 1 , pp. 37–52, 2017, [Online]. Available: https://sid.ir/paper/163285/en

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