RAW AND CALCINATION-MODIFIED COAL WASTE AS ADSORBENTS TO REMOVE CADMIUM FROM SIMULATED MINING WASTEWATER

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ZHANG M.; WANG H.

مرکز اطلاعات علمی Scientific Information Database (SID) - Trusted Source for Research and Academic Resources

Journal Paper

Paper Information

Journal: INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY (IJEST) Year:2014 | Volume:11 | Issue:4 Page(s): 987-996

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Information Journal Paper

Title

RAW AND CALCINATION-MODIFIED COAL WASTE AS ADSORBENTS TO REMOVE CADMIUM FROM SIMULATED MINING WASTEWATER

Author(s)

ZHANG M. | WANG H. | Issue Writer Certificate

Keywords

ADSORPTION

DESORPTION

HEAVY METAL

THERMODYNAMIC PARAMETERS

Abstract

The ADSORPTION of cadmium from simulated mining wastewater by coal waste (CW) and calcination-modified coal waste (MCW) was investigated. Effects of pH, initial concentration, particle size of adsorbent, adsorbent dosage and temperature were studied in batch experiments. The ADSORPTION efficiency for cadmium increased with increasing pH, and the optimum pH for cadmium ADSORPTION onto MCW and CW was 6.0 and 6.5, respectively. Kinetic experiments showed that the ADSORPTION equilibrium was reached within 120 min and followed pseudo-second-order model well. The ADSORPTION isotherm data fit Langmuir and Freundlich models, and the ADSORPTION capacity of cadmium on the two adsorbents increased with increasing temperature from 298 to 318 K. MCW had a higher ADSORPTION capacity of cadmium than CW, because calcination treatment can make CW to have more loose structure and higher specific surface area. THERMODYNAMIC PARAMETERS, the Gibbs free energy change (DG0), enthalpy change (DH0) and entropy change (DS0), were calculated and the results showed that the ADSORPTION of cadmium on CW and MCW was spontaneous and endothermic. Fourier transform infrared studies indicated silanol and aluminol groups were responsible for cadmium binding. The DESORPTION results indicated that the two adsorbents could be used repeatedly at least three times without significant decrease in the ADSORPTION capacity for cadmium. The results suggested that modified CW could have high potential as low-cost adsorbent for cadmium removal.

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APA: Copy

ZHANG, M., & WANG, H.. (2014). RAW AND CALCINATION-MODIFIED COAL WASTE AS ADSORBENTS TO REMOVE CADMIUM FROM SIMULATED MINING WASTEWATER. INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY (IJEST), 11(4), 987-996. SID. https://sid.ir/paper/285546/en

Vancouver: Copy

ZHANG M., WANG H.. RAW AND CALCINATION-MODIFIED COAL WASTE AS ADSORBENTS TO REMOVE CADMIUM FROM SIMULATED MINING WASTEWATER. INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY (IJEST)[Internet]. 2014;11(4):987-996. Available from: https://sid.ir/paper/285546/en

IEEE: Copy

M. ZHANG, and H. WANG, “RAW AND CALCINATION-MODIFIED COAL WASTE AS ADSORBENTS TO REMOVE CADMIUM FROM SIMULATED MINING WASTEWATER,” INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY (IJEST), vol. 11, no. 4, pp. 987–996, 2014, [Online]. Available: https://sid.ir/paper/285546/en

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