GRAPHENE OXIDE NANOSHEETS SUPPORTED MANGANESE (III) PORPHYRIN: A HIGHLY EFFICIENT AND REUSABLE BIOMIMETIC CATALYST FOR EPOXIDATION OF ALKENES WITH SODIUM PERIODATE

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ZARRINJAHAN ALIREZA; MOGHADDAM MAJID; MIRKHANI VALIOLLAH; TANGESTANINEJAD SHAHRAM; MOHAMMADPOUR BALTORK IRAJ

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Journal: JOURNAL OF THE IRANIAN CHEMICAL SOCIETY(JICS) Year:2016 | Volume:13 | Issue:8 Page(s): 0-0

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Title

GRAPHENE OXIDE NANOSHEETS SUPPORTED MANGANESE (III) PORPHYRIN: A HIGHLY EFFICIENT AND REUSABLE BIOMIMETIC CATALYST FOR EPOXIDATION OF ALKENES WITH SODIUM PERIODATE

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GRAPHENE OXIDE MANGANESE PORPHYR IN SUPPORTED CATALYST EPOXIDATION SODIUM PERIODATE

Abstract

Efficient epoxidation of alkenes catalyzed by tetrakis (p-aminophenyl) porphyrinato manganese (III) chloride, [Mn (TNH2PP) Cl], supported on graphene oxide nanosheets, is reported. The catalyst, [Mn (TNH2PP) Cl]@GO, was prepared by covalent attachment of amino groups of porphyrin to carboxylic acid groups of GO. This new heterogenized catalyst was characterized by ICP, FT-IR and diffuse reflectance UV–vis spectroscopies, scanning electron microscopy and transmission electron microscopy. This catalyst was applied as an efficient and reusable catalyst in the epoxidation of alkenes with NaIO4 at room temperature, in the presence of imidazole as axial ligand. The most noteworthy advantage of [Mn (TNH2PP)Cl]@GO is its high reusability in the oxidation reactions, in which the catalyst was reused several times without significant loss of its catalytic activity.

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APA: Copy

ZARRINJAHAN, ALIREZA, MOGHADDAM, MAJID, MIRKHANI, VALIOLLAH, TANGESTANINEJAD, SHAHRAM, & MOHAMMADPOUR BALTORK, IRAJ. (2016). GRAPHENE OXIDE NANOSHEETS SUPPORTED MANGANESE (III) PORPHYRIN: A HIGHLY EFFICIENT AND REUSABLE BIOMIMETIC CATALYST FOR EPOXIDATION OF ALKENES WITH SODIUM PERIODATE. JOURNAL OF THE IRANIAN CHEMICAL SOCIETY(JICS), 13(8), 0-0. SID. https://sid.ir/paper/283202/en

Vancouver: Copy

ZARRINJAHAN ALIREZA, MOGHADDAM MAJID, MIRKHANI VALIOLLAH, TANGESTANINEJAD SHAHRAM, MOHAMMADPOUR BALTORK IRAJ. GRAPHENE OXIDE NANOSHEETS SUPPORTED MANGANESE (III) PORPHYRIN: A HIGHLY EFFICIENT AND REUSABLE BIOMIMETIC CATALYST FOR EPOXIDATION OF ALKENES WITH SODIUM PERIODATE. JOURNAL OF THE IRANIAN CHEMICAL SOCIETY(JICS)[Internet]. 2016;13(8):0-0. Available from: https://sid.ir/paper/283202/en

IEEE: Copy

ALIREZA ZARRINJAHAN, MAJID MOGHADDAM, VALIOLLAH MIRKHANI, SHAHRAM TANGESTANINEJAD, and IRAJ MOHAMMADPOUR BALTORK, “GRAPHENE OXIDE NANOSHEETS SUPPORTED MANGANESE (III) PORPHYRIN: A HIGHLY EFFICIENT AND REUSABLE BIOMIMETIC CATALYST FOR EPOXIDATION OF ALKENES WITH SODIUM PERIODATE,” JOURNAL OF THE IRANIAN CHEMICAL SOCIETY(JICS), vol. 13, no. 8, pp. 0–0, 2016, [Online]. Available: https://sid.ir/paper/283202/en

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